2,11-Dimethoxyldipyridopurinone as an efficient reducing visible-light photocatalyst for organic transformations
文献情報
Yameng Wan, Qingfeng Liu, Hao Wu, Zhiguo Zhang, Guisheng Zhang
We report for the first time 2,11-dimethoxyldipyridopurinone (DP4) as a potent reducing visible-light photocatalyst toward three prototypic organic transformations: redox-neutral intramolecular aryltrifluoromethylations of acrylamides and the direct C–H arylation of heteroarenes with aryl diazonium salts, net oxidative hydroxylations of arylboronic acids using molecular oxygen as a green oxidant, and the net reductive dehalogenation/deuteration of α-bromocarbonyl compounds. This work reveals a bright future for dipyridopurinone derivatives as a new class of metal-free visible-light photocatalysts for a wide range of organic transformations.
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Organic Chemistry Frontiers
Organic Chemistry Frontiers publishes high-quality research from across organic chemistry. Emphases are placed on studies that make significant contributions to the field of organic chemistry by reporting either new or significantly improved protocols or methodologies. Topics include, but are not limited to the following: Organic synthesis Development of synthetic methodologies Catalysis Natural products Functional organic materials Supramolecular and macromolecular chemistry Physical and computational organic chemistry
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